螺旋磁性

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90K下锗化铁(FeGe)中螺旋自旋条纹的洛伦兹TEM图像

螺旋磁性是一种相邻磁矩的自旋以螺旋模式进行排列的磁序形式,其特征转角介于0到180度之间。这种现象是铁磁反铁磁交换相互作用之间竞争的结果,也可以分别将铁磁和反铁磁视为具有0度和180度特征转角的螺旋磁结构。螺旋磁序本质上可以是左旋或右旋的,因此螺旋磁序破坏了空间反演对称性

严格来说,螺旋磁体并没有永久磁矩,因此有时被认为是一种复杂的反铁磁体。而锥形磁性除了具有螺旋调制外还有永久磁矩(例如,金属钬在低于20K时表现出锥形磁性[1])。是否具有永久磁矩可以将螺旋磁体与锥形磁体区分开来。

螺旋磁性的概念于1959年首次提出,它可以作为对二氧化锰磁结构的解释[2]。螺旋磁性最初应用于中子衍射,后来发现它可以被洛伦兹电子显微镜更直接地观察到[3]。据报道,大部分材料在低温下表现出螺旋磁性,然而也有一些螺旋磁结构可以在室温下保持稳定[4]。许多螺旋磁体具有手性立方结构,例如B20晶体结构类型。

就像普通铁磁体具有分隔各个磁畴的畴壁一样,螺旋磁体也有自己的以拓扑电荷为特征的畴壁。 [5]

螺旋磁材料
材料 温度范围
β-MnO2 [2][6] < 93 K
FeGe, [4] < 278 K
MnGe[7] < 170 K
MnSi, [8] < 29 K
FexCo1−xSi (0.3 ≤ x ≤ 0.85) [9] [10]
Cu2OSeO3[11] < 58 K
Tb[12] 219–231 K
Dy[13] 85–179 K
Ho[14] 20–132 K

参见

参考文献

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  2. ^ 2.0 2.1 Yoshimori, Akio. A New Type of Antiferromagnetic Structure in the Rutile Type Crystal. Journal of the Physical Society of Japan (Physical Society of Japan). 1959, 14 (6): 807–821. Bibcode:1959JPSJ...14..807Y. doi:10.1143/jpsj.14.807. 
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  5. ^ Schoenherr, P.; Müller, J.; Köhler, L.; Rosch, A.; Kanazawa, N.; Tokura, Y.; Garst, M.; Meier, D. Topological domain walls in helimagnets. Nature Physics (Springer Science and Business Media LLC). 2018, 14 (5): 465–468. Bibcode:2018NatPh..14..465S. arXiv:1704.06288可免费查阅. doi:10.1038/s41567-018-0056-5. 
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